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|Title: ||One pot synthesis of higher order quasi-block copolymer libraries via sequential RAFT polymerization in an automated synthesizer|
|Authors: ||HAVEN, Joris|
Keddie, Daniel J.
Thang, San H.
Schubert, Ulrich S.
|Issue Date: ||2014|
|Publisher: ||ROYAL SOC CHEMISTRY|
|Citation: ||Polymer Chemistry, 5 (18), p. 5236-5246|
|Abstract: ||Recently developed sequential reversible addition-fragmentation chain transfer (RAFT) polymerization protocols allow the rapid, fully unattended preparation of quasi-block copolymer libraries that cover a wide range of copolymer compositions in an automated synthesizer. This contribution explores the scope and limitations of this sequential approach for the synthesis of higher order quasi-multiblock copolymers (including copolymer sequences of BAB, CBABC, ABC and ABCD). These syntheses illustrate the utility of this high-throughput approach for the one pot synthesis of functional polymers of increased complexity. Additionally, the use of this experimental technique for method development is highlighted.|
|Notes: ||[Haven, Joris J.; Guerrero-Sanchez, Carlos; Keddie, Daniel J.; Moad, Graeme; Thang, San H.] CSIRO, Clayton, Vic 3169, Australia. [Haven, Joris J.] Univ Hasselt, Inst Mat Res, Polymer React Design Grp, IMOMEC, B-3590 Diepenbeek, Belgium. [Guerrero-Sanchez, Carlos; Schubert, Ulrich S.] Univ Jena, Lab Organ & Macromol Chem IOMC, D-07743 Jena, Germany. [Guerrero-Sanchez, Carlos; Schubert, Ulrich S.] Univ Jena, JCSM, Polymer Libs, D-07743 Jena, Germany. [Keddie, Daniel J.] Univ New England, Chem Sch Sci & Technol, Armidale, NSW 2351, Australia.|
|ISI #: ||000340767100006|
|Type: ||Journal Contribution|
|Validation: ||ecoom, 2015|
|Appears in Collections: ||Research publications|
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